relation: http://publicatio.bibl.u-szeged.hu/29671/ title: Cooperative Self-Assembly in Linear Chains Based on Halogen Bonds creator: Vermeeren Pascal creator: Wolters Lando P. creator: Paragi Gábor creator: Fonseca Guerra Celia subject: 01.03. Fizikai tudományok description: Cooperative properties of halogen bonds were investigated with computational experiments based on dispersion-corrected relativistic density functional theory. The bonding mechanism in linear chains of cyanogen halide (X-CN), halocyanoacetylene (X-CC-CN), and 4-halobenzonitrile (X-C6H4-CN) were examined for X = H, Cl, Br, and I. Our energy decomposition and Kohn-Sham molecular-orbital analyses revealed the bonding mechanism of the studied systems. Cyanogen halide and halocyanoacetylene chains possess an extra stabilizing effect with increasing chain size, whereas the 4-halobenzonitrile chains do not. This cooperativity can be traced back to charge separation within the sigma-electronic system by charge-transfer between the lone-pair orbital of the nitrogen (sigma(HOMO)) on one unit and the acceptor orbital of the C-X (sigma*(LUMO)) on the adjacent unit. As such, the HOMO-LUMO gap in the sigma-system decreases, and the cooperativity increases with chain length revealing the similarity in the bonding mechanisms of hydrogen and halogen bonds. date: 2021 type: Folyóiratcikk type: PeerReviewed format: text identifier: http://publicatio.bibl.u-szeged.hu/29671/2/ChemPlusChem202186812-fulltext.pdf identifier: Vermeeren Pascal; Wolters Lando P.; Paragi Gábor; Fonseca Guerra Celia: Cooperative Self-Assembly in Linear Chains Based on Halogen Bonds. CHEMPLUSCHEM, 86 (6). pp. 812-819. ISSN 2192-6506 (2021) identifier: doi:10.1002/cplu.202100093 relation: https://doi.org/10.1002/cplu.202100093 relation: 32049042 language: eng